Suspended graphene device fabrication

Tämän pro gradu -tutkielman aiheena oli tutkia itsekantavien grafeeninäytteiden valmistusta. Grafeeni syntetisoitiin kaasufaasikasvatuksella ilmakehän paineessa kupariohutkalvoille. Kupariohutkalvot valmistattiin käyttämällä elektronisuihkuhöyrystystä. Projektin aikana synteesiprosessia parannettiin...

Full description

Bibliographic Details
Main Author: Hiltunen, Vesa-Matti
Other Authors: Matemaattis-luonnontieteellinen tiedekunta, Faculty of Sciences, Fysiikan laitos, Department of Physics, University of Jyväskylä, Jyväskylän yliopisto
Format: Master's thesis
Language:eng
Published: 2016
Subjects:
Online Access: https://jyx.jyu.fi/handle/123456789/49582
_version_ 1828193104589488128
author Hiltunen, Vesa-Matti
author2 Matemaattis-luonnontieteellinen tiedekunta Faculty of Sciences Fysiikan laitos Department of Physics University of Jyväskylä Jyväskylän yliopisto
author_facet Hiltunen, Vesa-Matti Matemaattis-luonnontieteellinen tiedekunta Faculty of Sciences Fysiikan laitos Department of Physics University of Jyväskylä Jyväskylän yliopisto Hiltunen, Vesa-Matti Matemaattis-luonnontieteellinen tiedekunta Faculty of Sciences Fysiikan laitos Department of Physics University of Jyväskylä Jyväskylän yliopisto
author_sort Hiltunen, Vesa-Matti
datasource_str_mv jyx
description Tämän pro gradu -tutkielman aiheena oli tutkia itsekantavien grafeeninäytteiden valmistusta. Grafeeni syntetisoitiin kaasufaasikasvatuksella ilmakehän paineessa kupariohutkalvoille. Kupariohutkalvot valmistattiin käyttämällä elektronisuihkuhöyrystystä. Projektin aikana synteesiprosessia parannettiin optimoimalla synteesiparametreja. Syntetisoinnin jälkeen grafeeninäytteet siirrettiin piinitridikalvoille, joihin oli valmistettu reikiä. Viimeinen vaihe siirrossa on PMMA tukikerroksen poisto grafeenin päältä, jota tutkittiin käyttämällä kahta eri menetelmää. Näistä ensimmäinen menetelmä oli lämpökäsittely ja toinen kriittisen pisteen kuivaus PMMA:n asetoniin liuottamisen jälkeen. Näytteet kuvannettiin käyttämällä pyyhkäisyelektronimikroskopiaa, läpäisyelektronimikroskopiaa sekä optista mikroskopiaa. Lisäksi näytteet karakterisoitiin käyttämällä Raman spektroskopiaa. Työn tuloksena alun synteesiongelmien jälkeen itsekantavaa grafeenia valmistettiin onnistuneesti. Eri PMMA:n poistomenetelmistä lämpökäsittely toimi monikerroksiselle grafeenille, mutta yksikerroksinen grafeeni ei selvinnyt käsittelystä. Kriittisen pisteen kuivaus toimi molemmissa tapauksissa, mutta jätti epäpuhtauksia, joten parhaaksi menetelmäksi selvisi PMMA: n poisto käyttämällä kriittisen pisteen kuivausta ja näytteiden puhdistus tämän jälkeen käyttämällä lämpökäsittelyä. In this Master’s thesis the production of suspended graphene devices was studied. Graphene was synthesized using atmospheric pressure chemical vapor deposition onto copper thin films that were fabricated using electron beam evaporation. During the project, the synthesis process was improved by optimizing synthesis parameters. After synthesis graphene samples were transferred onto silicon nitride membranes, which had openings fabricated to them. The last step of the transfer was removal of PMMA support layer from graphene, which was studied using two different methods. First of these was thermal annealing and the second critical point drying after dissolving the PMMA with acetone. Samples were imaged using scanning electron microscopy, transmission electron microscopy and optical microscopy. Further characterization was done with Raman spectroscopy. As for results, after some struggle with synthesis, suspended graphene was successfully fabricated. As for different PMMA cleaning methods, thermal annealing worked with multilayer graphene, but caused single layer graphene to break. Critical point drying worked in both cases, but left residues, so best method ended up being PMMA removal by critical point drying followed by cleaning of graphene by annealing.
first_indexed 2024-09-11T08:48:59Z
format Pro gradu
free_online_boolean 1
fullrecord [{"key": "dc.contributor.advisor", "value": "Johansson, Andreas", "language": null, "element": "contributor", "qualifier": "advisor", "schema": "dc"}, {"key": "dc.contributor.author", "value": "Hiltunen, Vesa-Matti", "language": null, "element": "contributor", "qualifier": "author", "schema": "dc"}, {"key": "dc.date.accessioned", "value": "2016-04-27T14:43:26Z", "language": null, "element": "date", "qualifier": "accessioned", "schema": "dc"}, {"key": "dc.date.available", "value": "2016-04-27T14:43:26Z", "language": null, "element": "date", "qualifier": "available", "schema": "dc"}, {"key": "dc.date.issued", "value": "2016", "language": null, "element": "date", "qualifier": "issued", "schema": "dc"}, {"key": "dc.identifier.other", "value": "oai:jykdok.linneanet.fi:1526482", "language": null, "element": "identifier", "qualifier": "other", "schema": "dc"}, {"key": "dc.identifier.uri", "value": "https://jyx.jyu.fi/handle/123456789/49582", "language": null, "element": "identifier", "qualifier": "uri", "schema": "dc"}, {"key": "dc.description.abstract", "value": "T\u00e4m\u00e4n pro gradu -tutkielman aiheena oli tutkia itsekantavien grafeenin\u00e4ytteiden\nvalmistusta. Grafeeni syntetisoitiin kaasufaasikasvatuksella ilmakeh\u00e4n paineessa kupariohutkalvoille.\nKupariohutkalvot valmistattiin k\u00e4ytt\u00e4m\u00e4ll\u00e4 elektronisuihkuh\u00f6yrystyst\u00e4.\nProjektin aikana synteesiprosessia parannettiin optimoimalla synteesiparametreja.\nSyntetisoinnin j\u00e4lkeen grafeenin\u00e4ytteet siirrettiin piinitridikalvoille, joihin oli\nvalmistettu reiki\u00e4. Viimeinen vaihe siirrossa on PMMA tukikerroksen poisto grafeenin\np\u00e4\u00e4lt\u00e4, jota tutkittiin k\u00e4ytt\u00e4m\u00e4ll\u00e4 kahta eri menetelm\u00e4\u00e4. N\u00e4ist\u00e4 ensimm\u00e4inen\nmenetelm\u00e4 oli l\u00e4mp\u00f6k\u00e4sittely ja toinen kriittisen pisteen kuivaus PMMA:n asetoniin\nliuottamisen j\u00e4lkeen. N\u00e4ytteet kuvannettiin k\u00e4ytt\u00e4m\u00e4ll\u00e4 pyyhk\u00e4isyelektronimikroskopiaa,\nl\u00e4p\u00e4isyelektronimikroskopiaa sek\u00e4 optista mikroskopiaa. Lis\u00e4ksi n\u00e4ytteet\nkarakterisoitiin k\u00e4ytt\u00e4m\u00e4ll\u00e4 Raman spektroskopiaa. Ty\u00f6n tuloksena alun synteesiongelmien\nj\u00e4lkeen itsekantavaa grafeenia valmistettiin onnistuneesti. Eri PMMA:n poistomenetelmist\u00e4\nl\u00e4mp\u00f6k\u00e4sittely toimi monikerroksiselle grafeenille, mutta yksikerroksinen\ngrafeeni ei selvinnyt k\u00e4sittelyst\u00e4. Kriittisen pisteen kuivaus toimi molemmissa\ntapauksissa, mutta j\u00e4tti ep\u00e4puhtauksia, joten parhaaksi menetelm\u00e4ksi selvisi PMMA:\nn poisto k\u00e4ytt\u00e4m\u00e4ll\u00e4 kriittisen pisteen kuivausta ja n\u00e4ytteiden puhdistus t\u00e4m\u00e4n\nj\u00e4lkeen k\u00e4ytt\u00e4m\u00e4ll\u00e4 l\u00e4mp\u00f6k\u00e4sittely\u00e4.", "language": "fi", "element": "description", "qualifier": "abstract", "schema": "dc"}, {"key": "dc.description.abstract", "value": "In this Master\u2019s thesis the production of suspended graphene devices was studied.\nGraphene was synthesized using atmospheric pressure chemical vapor deposition onto\ncopper thin films that were fabricated using electron beam evaporation. During the\nproject, the synthesis process was improved by optimizing synthesis parameters. After\nsynthesis graphene samples were transferred onto silicon nitride membranes, which\nhad openings fabricated to them. The last step of the transfer was removal of PMMA\nsupport layer from graphene, which was studied using two different methods. First\nof these was thermal annealing and the second critical point drying after dissolving\nthe PMMA with acetone. Samples were imaged using scanning electron microscopy,\ntransmission electron microscopy and optical microscopy. Further characterization\nwas done with Raman spectroscopy. As for results, after some struggle with synthesis,\nsuspended graphene was successfully fabricated. As for different PMMA cleaning\nmethods, thermal annealing worked with multilayer graphene, but caused single layer\ngraphene to break. Critical point drying worked in both cases, but left residues, so\nbest method ended up being PMMA removal by critical point drying followed by\ncleaning of graphene by annealing.", "language": "en", "element": "description", "qualifier": "abstract", "schema": "dc"}, {"key": "dc.description.provenance", "value": "Submitted using Plone Publishing form by Vesa-Matti Hiltunen (vejuhilt) on 2016-04-27 14:43:07.740084. Form: Pro gradu -lomake (https://kirjasto.jyu.fi/julkaisut/julkaisulomakkeet/pro-gradu-lomake). JyX data: [jyx_publishing-allowed (fi) =True]", "language": "en", "element": "description", "qualifier": "provenance", "schema": "dc"}, {"key": "dc.description.provenance", "value": "Submitted by jyx lomake-julkaisija (jyx-julkaisija.group@korppi.jyu.fi) on 2016-04-27T14:43:26Z\nNo. of bitstreams: 2\nURN:NBN:fi:jyu-201604272345.pdf: 159716838 bytes, checksum: 3eb5c0abbc98e1675e0c7b4e45d64de3 (MD5)\nlicense.html: 4805 bytes, checksum: 7aafd77c75764d2809df8b8ef8984448 (MD5)", "language": "en", "element": "description", "qualifier": "provenance", "schema": "dc"}, {"key": "dc.description.provenance", "value": "Made available in DSpace on 2016-04-27T14:43:26Z (GMT). No. of bitstreams: 2\nURN:NBN:fi:jyu-201604272345.pdf: 159716838 bytes, checksum: 3eb5c0abbc98e1675e0c7b4e45d64de3 (MD5)\nlicense.html: 4805 bytes, checksum: 7aafd77c75764d2809df8b8ef8984448 (MD5)\n Previous issue date: 2016", "language": "en", "element": "description", "qualifier": "provenance", "schema": "dc"}, {"key": "dc.format.extent", "value": "1 verkkoaineisto (66 s.)", "language": null, "element": "format", "qualifier": "extent", "schema": "dc"}, {"key": "dc.format.mimetype", "value": "application/pdf", "language": null, "element": "format", "qualifier": "mimetype", "schema": "dc"}, {"key": "dc.language.iso", "value": "eng", "language": null, "element": "language", "qualifier": "iso", "schema": "dc"}, {"key": "dc.rights", "value": "In Copyright", "language": "en", "element": "rights", "qualifier": null, "schema": "dc"}, {"key": "dc.subject.other", "value": "graphene", "language": null, "element": "subject", "qualifier": "other", "schema": "dc"}, {"key": "dc.subject.other", "value": "CVD", "language": null, "element": "subject", "qualifier": "other", "schema": "dc"}, {"key": "dc.subject.other", "value": "Raman spectroscopy", "language": null, "element": "subject", "qualifier": "other", "schema": "dc"}, {"key": "dc.subject.other", "value": "suspended graphene", "language": null, "element": "subject", "qualifier": "other", "schema": "dc"}, {"key": "dc.title", "value": "Suspended graphene device fabrication", "language": null, "element": "title", "qualifier": null, "schema": "dc"}, {"key": "dc.type", "value": "master thesis", "language": null, "element": "type", "qualifier": null, "schema": "dc"}, {"key": "dc.identifier.urn", "value": "URN:NBN:fi:jyu-201604272345", "language": null, "element": "identifier", "qualifier": "urn", "schema": "dc"}, {"key": "dc.type.ontasot", "value": "Pro gradu -tutkielma", "language": "fi", "element": "type", "qualifier": "ontasot", "schema": "dc"}, {"key": "dc.type.ontasot", "value": "Master\u2019s thesis", "language": "en", "element": "type", "qualifier": "ontasot", "schema": "dc"}, {"key": "dc.contributor.faculty", "value": "Matemaattis-luonnontieteellinen tiedekunta", "language": "fi", "element": "contributor", "qualifier": "faculty", "schema": "dc"}, {"key": "dc.contributor.faculty", "value": "Faculty of Sciences", "language": "en", "element": "contributor", "qualifier": "faculty", "schema": "dc"}, {"key": "dc.contributor.department", "value": "Fysiikan laitos", "language": "fi", "element": "contributor", "qualifier": "department", "schema": "dc"}, {"key": "dc.contributor.department", "value": "Department of Physics", "language": "en", "element": "contributor", "qualifier": "department", "schema": "dc"}, {"key": "dc.contributor.organization", "value": "University of Jyv\u00e4skyl\u00e4", "language": "en", "element": "contributor", "qualifier": "organization", "schema": "dc"}, {"key": "dc.contributor.organization", "value": "Jyv\u00e4skyl\u00e4n yliopisto", "language": "fi", "element": "contributor", "qualifier": "organization", "schema": "dc"}, {"key": "dc.subject.discipline", "value": "Soveltava fysiikka", "language": "fi", "element": "subject", "qualifier": "discipline", "schema": "dc"}, {"key": "dc.subject.discipline", "value": "Applied Physics", "language": "en", "element": "subject", "qualifier": "discipline", "schema": "dc"}, {"key": "dc.date.updated", "value": "2016-04-27T14:43:27Z", "language": null, "element": "date", "qualifier": "updated", "schema": "dc"}, {"key": "yvv.contractresearch.funding", "value": "0", "language": null, "element": "contractresearch", "qualifier": "funding", "schema": "yvv"}, {"key": "dc.type.coar", "value": "http://purl.org/coar/resource_type/c_bdcc", "language": null, "element": "type", "qualifier": "coar", "schema": "dc"}, {"key": "dc.rights.accesslevel", "value": "openAccess", "language": "fi", "element": "rights", "qualifier": "accesslevel", "schema": "dc"}, {"key": "dc.type.publication", "value": "masterThesis", "language": null, "element": "type", "qualifier": "publication", "schema": "dc"}, {"key": "dc.subject.oppiainekoodi", "value": "4023", "language": null, "element": "subject", "qualifier": "oppiainekoodi", "schema": "dc"}, {"key": "dc.subject.yso", "value": "grafeeni", "language": null, "element": "subject", "qualifier": "yso", "schema": "dc"}, {"key": "dc.subject.yso", "value": "ohutkalvot", "language": null, "element": "subject", "qualifier": "yso", "schema": "dc"}, {"key": "dc.format.content", "value": "fulltext", "language": null, "element": "format", "qualifier": "content", "schema": "dc"}, {"key": "dc.rights.url", "value": "https://rightsstatements.org/page/InC/1.0/", "language": null, "element": "rights", "qualifier": "url", "schema": "dc"}, {"key": "dc.type.okm", "value": "G2", "language": null, "element": "type", "qualifier": "okm", "schema": "dc"}]
id jyx.123456789_49582
language eng
last_indexed 2025-03-31T20:02:49Z
main_date 2016-01-01T00:00:00Z
main_date_str 2016
online_boolean 1
online_urls_str_mv {"url":"https:\/\/jyx.jyu.fi\/bitstreams\/64c57169-3ac0-4ed8-911b-1033877102f2\/download","text":"URN:NBN:fi:jyu-201604272345.pdf","source":"jyx","mediaType":"application\/pdf"}
publishDate 2016
record_format qdc
source_str_mv jyx
spellingShingle Hiltunen, Vesa-Matti Suspended graphene device fabrication graphene CVD Raman spectroscopy suspended graphene Soveltava fysiikka Applied Physics 4023 grafeeni ohutkalvot
title Suspended graphene device fabrication
title_full Suspended graphene device fabrication
title_fullStr Suspended graphene device fabrication Suspended graphene device fabrication
title_full_unstemmed Suspended graphene device fabrication Suspended graphene device fabrication
title_short Suspended graphene device fabrication
title_sort suspended graphene device fabrication
title_txtP Suspended graphene device fabrication
topic graphene CVD Raman spectroscopy suspended graphene Soveltava fysiikka Applied Physics 4023 grafeeni ohutkalvot
topic_facet 4023 Applied Physics CVD Raman spectroscopy Soveltava fysiikka grafeeni graphene ohutkalvot suspended graphene
url https://jyx.jyu.fi/handle/123456789/49582 http://www.urn.fi/URN:NBN:fi:jyu-201604272345
work_keys_str_mv AT hiltunenvesamatti suspendedgraphenedevicefabrication